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    Aqueous Phase Tracers of Chemical Weathering in a Semi-arid Mountain Critical Zone

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    Author
    Jardine, Angela Beth
    Issue Date
    2011
    Keywords
    aqueous chemistry
    catchment
    chemical weathering
    critical zone
    hydrologic controls
    rare earth elements
    Advisor
    Troch, Peter A
    Chorover, Jonathan D
    
    Metadata
    Show full item record
    Publisher
    The University of Arizona.
    Rights
    Copyright © is held by the author. Digital access to this material is made possible by the University Libraries, University of Arizona. Further transmission, reproduction or presentation (such as public display or performance) of protected items is prohibited except with permission of the author.
    Abstract
    Chemical weathering reactions are important for the physical, chemical, and biological development of the critical zone. We present findings from aqueous phase chemical analyses of surface and soil pore waters during a 15 month study in a small semi-arid mountain catchment of the Santa Catalina Mountain Critical Zone Observatory. Stream water geochemical solutes are sourced to two distinct locations - fractured bedrock baseflow stores and soil quickflow stores. Solid phase observations of albite, anorthite, and K-feldspar transformation to Ca-montmorillonite and kaolinite are supported by stream water saturation states calculated via a PHREEQC geochemical model. While differences in mineral assemblages, soil depths, and horizonation suggest greater weathering in schist versus granite lithologies and in hillslope divergent versus convergent zones, soil pore water solute ratio analysis does not readily distinguish these differences. However, preliminary investigation of aqueous rare earth elements suggests detectable lithologic and landscape positional differences warranting focus for future research efforts.
    Type
    Electronic Thesis
    text
    Degree Name
    M.S.
    Degree Level
    masters
    Degree Program
    Graduate College
    Hydrology
    Degree Grantor
    University of Arizona
    Collections
    Master's Theses

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