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dc.contributor.authorBahl, A.
dc.contributor.authorWright, E. M.
dc.contributor.authorKolesik, M.
dc.date.accessioned2016-12-02T00:54:18Z
dc.date.available2016-12-02T00:54:18Z
dc.date.issued2016-08-29
dc.identifier.citationNonlinear optical response of noble gases via the metastable electronic state approach 2016, 94 (2) Physical Review Aen
dc.identifier.issn2469-9926
dc.identifier.issn2469-9934
dc.identifier.doi10.1103/PhysRevA.94.023850
dc.identifier.urihttp://hdl.handle.net/10150/621484
dc.description.abstractThe goal of this paper is to elucidate the theoretical underpinnings of the metastable electronic state approach (MESA) and demonstrate its utility for the evaluation of the nonlinear optical response of noble-gas atoms with emphasis on the application of the method to the propagation of multicolor optical fields in large-scale, spatially resolved simulations. More specifically, single-active-electron models of various atoms are employed to calculate their nonlinear properties both within the adiabatic approximation, involving a single metastable state and beyond, capturing inertial effects, and wavelength-dependent ionization. Simulations for excitation pulses at different center wavelengths as well as ionization in two-color pulses are presented and compared with numerical solutions of the time-dependent Schrodinger equation. Illustrative examples of the numerical simulation of high-power pulse propagation incorporating MESA data are also presented and showcase the successful application to optical filamentation in the midinfrared region.
dc.description.sponsorshipAir Force Office of Scientific Research [FA9550-16-1-0121, FA9550-13-1-0228]en
dc.language.isoenen
dc.publisherAMER PHYSICAL SOCen
dc.relation.urlhttp://link.aps.org/doi/10.1103/PhysRevA.94.023850en
dc.rights©2016 American Physical Societyen
dc.titleNonlinear optical response of noble gases via the metastable electronic state approachen
dc.typeArticleen
dc.contributor.departmentUniv Arizona, Coll Opt Scien
dc.identifier.journalPhysical Review Aen
dc.description.collectioninformationThis item from the UA Faculty Publications collection is made available by the University of Arizona with support from the University of Arizona Libraries. If you have questions, please contact us at repository@u.library.arizona.edu.en
dc.eprint.versionFinal published versionen
refterms.dateFOA2018-09-11T15:58:47Z
html.description.abstractThe goal of this paper is to elucidate the theoretical underpinnings of the metastable electronic state approach (MESA) and demonstrate its utility for the evaluation of the nonlinear optical response of noble-gas atoms with emphasis on the application of the method to the propagation of multicolor optical fields in large-scale, spatially resolved simulations. More specifically, single-active-electron models of various atoms are employed to calculate their nonlinear properties both within the adiabatic approximation, involving a single metastable state and beyond, capturing inertial effects, and wavelength-dependent ionization. Simulations for excitation pulses at different center wavelengths as well as ionization in two-color pulses are presented and compared with numerical solutions of the time-dependent Schrodinger equation. Illustrative examples of the numerical simulation of high-power pulse propagation incorporating MESA data are also presented and showcase the successful application to optical filamentation in the midinfrared region.


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