Analysis of aerosol composition data for western United States wildfires between 2005 and 2015: Dust emissions, chloride depletion, and most enhanced aerosol constituents
AuthorSchlosser, Joseph S.
Braun, Rachel A.
MacDonald, Alexander B.
Aldhaif, Abdulmonam A.
Aghdam, Mojtaba Azadi
Mardi, Ali Hossein
AffiliationUniv Arizona, Dept Chem & Environm Engn
Univ Arizona, Dept Hydrol & Atmospher Sci
MetadataShow full item record
PublisherAMER GEOPHYSICAL UNION
CitationAnalysis of aerosol composition data for western United States wildfires between 2005 and 2015: Dust emissions, chloride depletion, and most enhanced aerosol constituents 2017, 122 (16):8951 Journal of Geophysical Research: Atmospheres
Rights© 2017. American Geophysical Union. All Rights Reserved.
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AbstractThis study examines major wildfires in the western United States between 2005 and 2015 to determine which species exhibit the highest percent change in mass concentration on day of peak fire influence relative to preceding nonfire days. Forty-one fires were examined using the Environmental Protection Agency (EPA) Interagency Monitoring of Protected Visual Environments (IMPROVE) data set. Organic carbon (OC) and elemental carbon (EC) constituents exhibited the highest percent change increase. The sharpest enhancements were for the volatile (OC1) and semivolatile (OC2) OC fractions, suggestive of secondary organic aerosol formation during plume transport. Of the noncarbonaceous constituents, Cl, P, K, NO3-, and Zn levels exhibited the highest percent change. Dust was significantly enhanced in wildfire plumes, based on significant enhancements in fine soil components (i.e., Si, Ca, Al, Fe, and Ti) and PMcoarse (i.e., PM10-PM2.5). A case study emphasized how transport of wildfire plumes significantly impacted downwind states, with higher levels of fine soil and PMcoarse at the downwind state (Arizona) as compared to the source of the fires (California). A global model (Navy Aerosol Analysis and Prediction System, NAAPS) did not capture the dust influence over California or Arizona during this case event because it is not designed to resolve dust dynamics in fires, which motivates improved treatment of such processes. Significant chloride depletion was observed on the peak EC day for almost a half of the fires examined. Size-resolved measurements during two specific fires at a coastal California site revealed significant chloride reductions for particle aerodynamic diameters between 1 and 10 mu m.
Note6 month embargo; published online: 27 Aug 2017.
VersionFinal published version
SponsorsNational Institute of Environmental Health Sciences (NIEHS) Superfund Research Program [2 P42 ES04940]; ONR [N00014-16-1-2567, N00014-10-1-0811]; NASA/HQ; Agilent Technologies; U.S. Environmental Protection Agency; National Park Service
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