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    Short-range magnetic correlations in quasicrystalline i -Tb-Cd

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    PhysRevB.108.134421.pdf
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    Author
    Das, P.
    Kreyssig, A.
    Tucker, G.S.
    Podlesnyak, A.
    Ye, F.
    Matsuda, M.
    Kong, T.
    Bud'Ko, S.L.
    Canfield, P.C.
    Flint, R.
    Orth, P.P.
    Yamada, T.
    McQueeney, R.J.
    Goldman, A.I.
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    Affiliation
    Department of Physics, University of Arizona
    Issue Date
    2023-10-17
    
    Metadata
    Show full item record
    Publisher
    American Physical Society
    Citation
    P. Das, A. Kreyssig, G. S. Tucker, A. Podlesnyak, Feng Ye, Masaaki Matsuda, T. Kong, S. L. Bud'ko, P. C. Canfield, R. Flint, P. P. Orth, T. Yamada, R. J. McQueeney, and A. I. Goldman Phys. Rev. B 108, 134421 – Published 17 October 2023
    Journal
    Physical Review B
    Rights
    © 2023 American Physical Society.
    Collection Information
    This item from the UA Faculty Publications collection is made available by the University of Arizona with support from the University of Arizona Libraries. If you have questions, please contact us at repository@u.library.arizona.edu.
    Abstract
    We report on elastic and inelastic neutron scattering from single-grain isotopically enriched samples to elucidate the local magnetic correlations between Tb3+ moments in quasicrystalline i-Tb-Cd. The inelastic neutron scattering measurements of the crystalline electric field excitations demonstrated that the Tb3+ moments are directed primarily along the local fivefold axes of the Tsai-type cluster as was found for the TbCd6 approximant phase. Based on the inelastic measurements, we consider a simple Ising-type model for the moment configurations on a single Tb3+ icosahedron and enumerate the lowest energy moment configurations. We then calculate the diffuse scattering from these configurations and compare with the experimental magnetic diffuse scattering measurements to identify the most likely single cluster moment configurations and find reasonable agreement between the broad features observed in our scattering simulations. We further use a heuristic glass model as well as large-scale Monte-Carlo simulations of a multicluster model to consider the role of higher-order (longer-range) intercluster correlations for magnetic frustration and the magnetic scattering. © 2023 American Physical Society.
    Note
    Immediate access
    ISSN
    2469-9950
    DOI
    10.1103/PhysRevB.108.134421
    Version
    Final Published Version
    ae974a485f413a2113503eed53cd6c53
    10.1103/PhysRevB.108.134421
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